CASTLE

See project website: https://www.castle.unifi.it/


 

 

Team at UNIPR, sQS group

  1. Stefano Carretta: Principal Investigator.
  2. Paolo Santini: Full Professor. Microscopic Models for CISS in Electron Transfer.
  3. Roberto De Renzi: Full Professor. Nuclear Magnetic Resonance and muon spin resonance experiments on chiral molecules to unveil CISS.
  4. Giuseppe Allodi: Associate Professor. Nuclear Magnetic Resonance and muon spin resonance experiments on chiral molecules to unveil CISS.
  5. Alessandro Chiesa: Research Associate. Theoretical models for CISS in Electron Transfer. Design of applications exploiting CISS for quantum technologies. Design and interpretation of time-resolved Electron Paramagnetic Resonance and Nuclear Mganetic Resonance experiments to unravel CISS.
  6. Elena Garlatti: Research Associate. Models for CISS in Electron Transfer starting from ab-initio calculations. Design and interpretation of experiments showing CISS in electron-transfer.
  7. Pietro Bonfà: Research Associate. First-principles calculations based on density-functional theory on chiral molecules to derive parameters for a microscopic model of CISS in electron transfer.
  8. Leonardo Celada: PhD student. Models for CISS in transport and electron-trasfer setups. 
  9. Arianna Cantarella: PhD student. First-principles calculations on chiral molecules displying CISS effect.

Research lines

  • Electron-transfer and chirality
  • Intramolecular CISS
  • CISS & qubit control
  • CISS and quantum enabled technologies

Research tools at UNIPR, sQS group

  • Theory: development of a microscopic model to understand the origin of CISS in electron transfer processes.
  • Interpretation of experiments unravelling CISS, in particular time-resolved electron paramagnetic resonance (trEPR).
  • Design, development and interpretation of novel experiments to unveil CISS in electron transfer, exploiting in particular nuclear spins as a probe.
  • Design of applications for quantum technologies and of proof-of-principle experiments.

Publications

  1. A. Chiesa, P. Santini, E. Garlatti, F. Luis, and S. Carretta, Molecular Nanomagnets: a viable path toward quantum information processing? Rep. Progr. Phys. 87, 034501 (2024).
  2. H. J. Eckvahl,* N. A. Tcyrulnikov,* A. Chiesa,* J. M. Bradley, R. M. Young, S. Carretta, M. D. Krzyaniak, M. R. Wasielewski, Direct Observation of Chirality-Induced Spin Selectivity in Electron Donor-Acceptor Molecules, Science 382, 197-201 (2023).
  3. E. Macaluso, A. Chiesa, P. Santini, R. Bittl, S. Carretta, Chiral-Induced Spin Selectivity in Photo-Induced Electron Transfer: investigating charge and spin dynamics in a master equation framework, J. Chem. Phys. 159, 084301 (2023).
  4. A. Chiesa, A. Privitera, E. Macaluso, M. Mannini, R. Bittl, R. Naaman, M. Wasielewski, R. Sessoli, S. Carretta, Chirality-induced spin selectivity: an enabling technology for quantum applications, Adv. Mater. 35, 2300472 (2023).

Conferences

  • S. Carretta, “Molecular Spin Qudits and Chiral-Induced Spin Selectivity: two promising tools for Quantum Technologies”, invited talk at the workshop Electron spin for quantum technologies: from molecules to devices, Turin, May 19th 2023.
  • S. Carretta, “Molecular Spin Qubits and Chiral-Induced Spin Selectivity: Two Promising Tools for Quantum Technologies”, invited talk at Copenhagen Molecular Quantum Information Discussions, Copenhagen, June 28th – 30th  2023.
  • A. Chiesa, "Chirality-Induced Spin Selectivity: An Enabling Technology for Quantum Applications", July 20th 2023, invited talk at the KUJI QMAT Online Journal Club (online).
  • S. Carretta, “Molecular Spin Qubits and Chiral-Induced Spin Selectivity: Two Promising Tools for Quantum Technologies”, invited talk at the ACS fall meeting, August 21st 2023.
  • A. Chiesa, "Chirality-Induced Spin Selectivity: An Enabling Technology for Quantum Applications", invited talk at 30th Condensed Matter Division and FisMat joint Conference, Milan, September 4th-8th 2023. 
  • S. Carretta, “Molecular Spin Qubits and Chiral-Induced Spin Selectivity: Two Promising Tools for Quantum Technologies”, invited talk at the 18th IEEE Nanotechnology Materials and Devices Conference (NMDC 2023), Paestum, October 22nd-25th, 2023.
  • A. Chiesa, "Chirality-Induced Spin Selectivity: An Enabling Technology for Quantum Applications", talk at the 5th Chirality@The Nanoscale conference, Angers, October 1st-5th 2023.
  • S. Carretta, "Molecular Spin Qubits and Chiral-Induced Spin Selectivity: Two Promising Tools for Quantum Technologies", invited talk at Spin meeting, Manchester, January 10th-12th 2024.
  • A. Chiesa, "Chirality-Induced Spin Selectivity in Electron Donor-Acceptor molecules:a resource for Quantum Technologies", talk at the 8th Italian Conference on Magnetism MAGNET2024, Milan, February 7th-9th 2024.